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J. Semicond. > 2020, Volume 41?>?Issue 9?> 090401

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A close step towards industrialized application of solar water splitting

Jun Liu^{1, 2}, Zhijie Wang^{1, 2,} and Yong Lei^3,

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• 1. Key Laboratory of Semiconductor Materials Science, Beijing Key Laboratory of Low Dimensional Semiconductor Materials and Devices, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, ChinaKey Laboratory of Semiconductor Materials Science, Beijing Key Laboratory of Low Dimensional Semiconductor Materials and Devices, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, China
• 2. Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, ChinaCenter of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
• 3. Institut für Physik & IMN MacroNano? (ZIK), Technische Universit?t Ilmenau, Ilmenau 98693, GermanyInstitut für Physik & IMN MacroNano? (ZIK), Technische Universit?t Ilmenau, Ilmenau 98693, Germany

• Jun Liu
• Zhijie Wang
• Yong Lei

 Corresponding author: Z Wang, wangzj@semi.ac.cn; Y Lei, yong.lei@tu-ilmenau.de

DOI: 10.1088/1674-4926/41/9/090401

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References

[1]	Fujishima A, Honda K. Electrochemical photolysis of water at a semiconductor electrode. Nature, 1972, 238, 37 doi: 10.1038/238037a0
[2]	An X, Li T, Wen B, et al. New insights into defect-mediated heterostructures for photoelectrochemical water splitting. Adv Energy Mater, 2016, 6, 1502268 doi: 10.1002/aenm.201502268
[3]	Wang X D, Xu Y F, Rao H S, et al. Novel porous molybdenum tungsten phosphide hybrid nanosheets on carbon cloth for efficient hydrogen evolution. Energ Environ Sci, 2016, 9, 1468 doi: 10.1039/C5EE03801D
[4]	Wu B, Liu D, Mubeen S, et al. Anisotropic growth of TiO2 onto gold nanorods for plasmon-enhanced hydrogen production from water reduction. J Am Chem Soc, 2016, 138, 1114 doi: 10.1021/jacs.5b11341
[5]	Zhang L, Ye X, Boloor M, et al. Significantly enhanced photocurrent for water oxidation in monolithic Mo:BiVO4/SnO2/Si by thermally increasing the minority carrier diffusion length. Energ Environ Sci, 2016, 9, 2044 doi: 10.1039/C6EE00036C
[6]	Luo J, Steier L, Son M K, et al. Cu2O nanowire photocathodes for efficient and durable solar water splitting. Nano Lett, 2016, 16, 1848 doi: 10.1021/acs.nanolett.5b04929
[7]	Domen K, Naito S, Soma M, et al. Photocatalytic decomposition of water vapour on an NiO–SrTiO3 catalyst. J Chem Soc Chem Commun, 1980, 12, 543 doi: 10.1039/c39800000543
[8]	Zou Z, Ye J, Sayama K, et al. Direct splitting of water under visible light irradiation with an oxide semiconductor photocatalyst. Nature, 2001, 414, 625 doi: 10.1038/414625a
[9]	Maeda K, Takata T, Hara M, et al. GaN:ZnO solid solution as a photocatalyst for visible-light-driven overall water splitting. J Am Chem Soc, 2005, 127, 8286 doi: 10.1021/ja0518777
[10]	Liu J, Liu Y, Liu N, et al. Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway. Science, 2015, 347, 970 doi: 10.1126/science.aaa3145
[11]	Takata T, Jiang J, Sakata Y, et al. Photocatalytic water splitting with a quantum efficiency of almost unity. Nature, 2020, 581, 411 doi: 10.1038/s41586-020-2278-9
[12]	Maeda K, Domen K. Photocatalytic water eplitting: Recent progress and future challenges. J Phys Chem Lett, 2010, 1, 2655 doi: 10.1021/jz1007966
[13]	Wang Z, Inoue Y, Hisatomi T, et al. Overall water splitting by Ta3N5 nanorod single crystals grown on the edges of KTaO3 particles. Nat Catal, 2018, 1, 756 doi: 10.1038/s41929-018-0134-1
[14]	Wang Q, Nakabayashi M, Hisatomi T, et al. Oxysulfide photocatalyst for visible-light-driven overall water splitting. Nat Mater, 2019, 18, 827 doi: 10.1038/s41563-019-0399-z

Fig. 1.  Photocatalytic water-splitting activities. (a) Time course of H₂ and O₂ evolution on SrTiO₃:Al loaded with various cocatalysts during photoirradiation. Left, loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%) by two-step photodeposition. Middle, loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%) by three-step photodeposition. Right, loaded with Rh (0.1 wt%)-Cr (0.1 wt%) oxide by co-impregnation. (b) Ultraviolet-visible diffuse reflectance spectrum of bare SrTiO₃:Al (black solid line) and wavelength dependence of external quantum efficiency (EQE) during water splitting on Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%)-loaded SrTiO₃:Al (red symbols).

DownLoad: Full-Size Img PowerPoint

Fig. 2.  Transmission electron microscopy. (a) Selected-area electron diffraction pattern obtained from SrTiO₃:Al loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%). (b) Corresponding transmission electron microscopy image of a particle. (c) Particle morphology and crystal orientation.

DownLoad: Full-Size Img PowerPoint

Fig. 3.  Simulations of photocarrier distributions in SrTiO₃:Al particles. (a) Mapping of conduction-band energy, E_c. (b) Density of electrons (e^-), n. (c) Density of holes (h⁺), p. (d) Energy band diagram. (e) Electron and hole densities as functions of position (x′, y′) with work function difference ΔW_el = 0.2 eV. (f) Effect of ΔW_el on electron-to-hole-density ratio at the {100} and {110} facets.

DownLoad: Full-Size Img PowerPoint

[1]	Fujishima A, Honda K. Electrochemical photolysis of water at a semiconductor electrode. Nature, 1972, 238, 37 doi: 10.1038/238037a0
[2]	An X, Li T, Wen B, et al. New insights into defect-mediated heterostructures for photoelectrochemical water splitting. Adv Energy Mater, 2016, 6, 1502268 doi: 10.1002/aenm.201502268
[3]	Wang X D, Xu Y F, Rao H S, et al. Novel porous molybdenum tungsten phosphide hybrid nanosheets on carbon cloth for efficient hydrogen evolution. Energ Environ Sci, 2016, 9, 1468 doi: 10.1039/C5EE03801D
[4]	Wu B, Liu D, Mubeen S, et al. Anisotropic growth of TiO2 onto gold nanorods for plasmon-enhanced hydrogen production from water reduction. J Am Chem Soc, 2016, 138, 1114 doi: 10.1021/jacs.5b11341
[5]	Zhang L, Ye X, Boloor M, et al. Significantly enhanced photocurrent for water oxidation in monolithic Mo:BiVO4/SnO2/Si by thermally increasing the minority carrier diffusion length. Energ Environ Sci, 2016, 9, 2044 doi: 10.1039/C6EE00036C
[6]	Luo J, Steier L, Son M K, et al. Cu2O nanowire photocathodes for efficient and durable solar water splitting. Nano Lett, 2016, 16, 1848 doi: 10.1021/acs.nanolett.5b04929
[7]	Domen K, Naito S, Soma M, et al. Photocatalytic decomposition of water vapour on an NiO–SrTiO3 catalyst. J Chem Soc Chem Commun, 1980, 12, 543 doi: 10.1039/c39800000543
[8]	Zou Z, Ye J, Sayama K, et al. Direct splitting of water under visible light irradiation with an oxide semiconductor photocatalyst. Nature, 2001, 414, 625 doi: 10.1038/414625a
[9]	Maeda K, Takata T, Hara M, et al. GaN:ZnO solid solution as a photocatalyst for visible-light-driven overall water splitting. J Am Chem Soc, 2005, 127, 8286 doi: 10.1021/ja0518777
[10]	Liu J, Liu Y, Liu N, et al. Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway. Science, 2015, 347, 970 doi: 10.1126/science.aaa3145
[11]	Takata T, Jiang J, Sakata Y, et al. Photocatalytic water splitting with a quantum efficiency of almost unity. Nature, 2020, 581, 411 doi: 10.1038/s41586-020-2278-9
[12]	Maeda K, Domen K. Photocatalytic water eplitting: Recent progress and future challenges. J Phys Chem Lett, 2010, 1, 2655 doi: 10.1021/jz1007966
[13]	Wang Z, Inoue Y, Hisatomi T, et al. Overall water splitting by Ta3N5 nanorod single crystals grown on the edges of KTaO3 particles. Nat Catal, 2018, 1, 756 doi: 10.1038/s41929-018-0134-1
[14]	Wang Q, Nakabayashi M, Hisatomi T, et al. Oxysulfide photocatalyst for visible-light-driven overall water splitting. Nat Mater, 2019, 18, 827 doi: 10.1038/s41563-019-0399-z

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Received: Revised: Online: Accepted Manuscript: 13 August 2020Uncorrected proof: 18 August 2020Published: 04 September 2020

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Article Navigation >  Journal of Semiconductors  > 2020  >  41(9): 090401

Jun Liu, Zhijie Wang, Yong Lei. A close step towards industrialized application of solar water splitting[J]. Journal of Semiconductors, 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401 ****J Liu, Z J Wang, Y Lei, A close step towards industrialized application of solar water splitting[J]. J. Semicond., 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401.

Citation:

Jun Liu, Zhijie Wang, Yong Lei. A close step towards industrialized application of solar water splitting[J]. Journal of Semiconductors, 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401 **** J Liu, Z J Wang, Y Lei, A close step towards industrialized application of solar water splitting[J]. J. Semicond., 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401.

Jun Liu, Zhijie Wang, Yong Lei. A close step towards industrialized application of solar water splitting[J]. Journal of Semiconductors, 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401 ****J Liu, Z J Wang, Y Lei, A close step towards industrialized application of solar water splitting[J]. J. Semicond., 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401.

Citation:

Jun Liu, Zhijie Wang, Yong Lei. A close step towards industrialized application of solar water splitting[J]. Journal of Semiconductors, 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401 **** J Liu, Z J Wang, Y Lei, A close step towards industrialized application of solar water splitting[J]. J. Semicond., 2020, 41(9): 090401. doi: 10.1088/1674-4926/41/9/090401.

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A close step towards industrialized application of solar water splitting

DOI: 10.1088/1674-4926/41/9/090401

• Jun Liu^1,2, 
• Zhijie Wang^1,2,  , 
• Yong Lei^3, 

• 1.

  Key Laboratory of Semiconductor Materials Science, Beijing Key Laboratory of Low Dimensional Semiconductor Materials and Devices, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, China

• 2.

  Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

• 3.

  Institut für Physik & IMN MacroNano? (ZIK), Technische Universit?t Ilmenau, Ilmenau 98693, Germany

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• Corresponding author: Z Wang, wangzj@semi.ac.cn; Y Lei, yong.lei@tu-ilmenau.de
• Published Date: 2020-09-10

Abstract
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References(14)

• References

  [1]	Fujishima A, Honda K. Electrochemical photolysis of water at a semiconductor electrode. Nature, 1972, 238, 37 doi: 10.1038/238037a0
  [2]	An X, Li T, Wen B, et al. New insights into defect-mediated heterostructures for photoelectrochemical water splitting. Adv Energy Mater, 2016, 6, 1502268 doi: 10.1002/aenm.201502268
  [3]	Wang X D, Xu Y F, Rao H S, et al. Novel porous molybdenum tungsten phosphide hybrid nanosheets on carbon cloth for efficient hydrogen evolution. Energ Environ Sci, 2016, 9, 1468 doi: 10.1039/C5EE03801D
  [4]	Wu B, Liu D, Mubeen S, et al. Anisotropic growth of TiO2 onto gold nanorods for plasmon-enhanced hydrogen production from water reduction. J Am Chem Soc, 2016, 138, 1114 doi: 10.1021/jacs.5b11341
  [5]	Zhang L, Ye X, Boloor M, et al. Significantly enhanced photocurrent for water oxidation in monolithic Mo:BiVO4/SnO2/Si by thermally increasing the minority carrier diffusion length. Energ Environ Sci, 2016, 9, 2044 doi: 10.1039/C6EE00036C
  [6]	Luo J, Steier L, Son M K, et al. Cu2O nanowire photocathodes for efficient and durable solar water splitting. Nano Lett, 2016, 16, 1848 doi: 10.1021/acs.nanolett.5b04929
  [7]	Domen K, Naito S, Soma M, et al. Photocatalytic decomposition of water vapour on an NiO–SrTiO3 catalyst. J Chem Soc Chem Commun, 1980, 12, 543 doi: 10.1039/c39800000543
  [8]	Zou Z, Ye J, Sayama K, et al. Direct splitting of water under visible light irradiation with an oxide semiconductor photocatalyst. Nature, 2001, 414, 625 doi: 10.1038/414625a
  [9]	Maeda K, Takata T, Hara M, et al. GaN:ZnO solid solution as a photocatalyst for visible-light-driven overall water splitting. J Am Chem Soc, 2005, 127, 8286 doi: 10.1021/ja0518777
  [10]	Liu J, Liu Y, Liu N, et al. Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway. Science, 2015, 347, 970 doi: 10.1126/science.aaa3145
  [11]	Takata T, Jiang J, Sakata Y, et al. Photocatalytic water splitting with a quantum efficiency of almost unity. Nature, 2020, 581, 411 doi: 10.1038/s41586-020-2278-9
  [12]	Maeda K, Domen K. Photocatalytic water eplitting: Recent progress and future challenges. J Phys Chem Lett, 2010, 1, 2655 doi: 10.1021/jz1007966
  [13]	Wang Z, Inoue Y, Hisatomi T, et al. Overall water splitting by Ta3N5 nanorod single crystals grown on the edges of KTaO3 particles. Nat Catal, 2018, 1, 756 doi: 10.1038/s41929-018-0134-1
  [14]	Wang Q, Nakabayashi M, Hisatomi T, et al. Oxysulfide photocatalyst for visible-light-driven overall water splitting. Nat Mater, 2019, 18, 827 doi: 10.1038/s41563-019-0399-z

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• Fig. 1. Photocatalytic water-splitting activities. (a) Time course of H₂ and O₂ evolution on SrTiO₃:Al loaded with various cocatalysts during photoirradiation. Left, loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%) by two-step photodeposition. Middle, loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%) by three-step photodeposition. Right, loaded with Rh (0.1 wt%)-Cr (0.1 wt%) oxide by co-impregnation. (b) Ultraviolet-visible diffuse reflectance spectrum of bare SrTiO₃:Al (black solid line) and wavelength dependence of external quantum efficiency (EQE) during water splitting on Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%)-loaded SrTiO₃:Al (red symbols).
• Fig. 2. Transmission electron microscopy. (a) Selected-area electron diffraction pattern obtained from SrTiO₃:Al loaded with Rh (0.1 wt%)/Cr₂O₃ (0.05 wt%)/CoOOH (0.05 wt%). (b) Corresponding transmission electron microscopy image of a particle. (c) Particle morphology and crystal orientation.
• Fig. 3. Simulations of photocarrier distributions in SrTiO₃:Al particles. (a) Mapping of conduction-band energy, E_c. (b) Density of electrons (e^-), n. (c) Density of holes (h⁺), p. (d) Energy band diagram. (e) Electron and hole densities as functions of position (x′, y′) with work function difference ΔW_el = 0.2 eV. (f) Effect of ΔW_el on electron-to-hole-density ratio at the {100} and {110} facets.